Characterizing the Biosynthesis of the [Fe(II)(CN)(CO)2(cysteinate)]- Organometallic Product of the Radical-SAM Enzyme HydG by EPR and Mossbauer Spectroscopy

Villarreal, DG; Rao, GD; Tao, LZ; Liu, L; Rauchfuss, TB; Britt, RD

Britt, RD (通讯作者)，Univ Calif Davis, Dept Chem, Davis, CA 95616 USA.

JOURNAL OF PHYSICAL CHEMISTRY B, 2023; 127 (43): 9295

Abstract

[FeFe]-hydrogenases employ a catalytic H-cluster, consisting of a [4Fe-4S](H) cluster linked to a [2Fe](H) subcluster with CO, CN- ligands, and an aza......

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